Determination of persimmon leaf chloride contents using near-infrared spectroscopy (NIRS)

Early diagnosis of specific chloride toxicity in persimmon trees requires the reliable and fast determination of the leaf chloride content, which is usually performed by means of a cumbersome, expensive and time-consuming wet analysis. A methodology has been developed in this study as an alternative...

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Autores principales: De-Paz, José M., Visconti, Fernando, Chiaravalle, Mara, Quinones, Ana
Formato: publishedVersion
Lenguaje:Inglés
Publicado: Springer Verlag 2020
Materias:
Acceso en línea:http://hdl.handle.net/20.500.11939/6587
https://link.springer.com/article/10.1007%2Fs00216-016-9430-2
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author De-Paz, José M.
Visconti, Fernando
Chiaravalle, Mara
Quinones, Ana
author_browse Chiaravalle, Mara
De-Paz, José M.
Quinones, Ana
Visconti, Fernando
author_facet De-Paz, José M.
Visconti, Fernando
Chiaravalle, Mara
Quinones, Ana
author_sort De-Paz, José M.
collection ReDivia
description Early diagnosis of specific chloride toxicity in persimmon trees requires the reliable and fast determination of the leaf chloride content, which is usually performed by means of a cumbersome, expensive and time-consuming wet analysis. A methodology has been developed in this study as an alternative to determine chloride in persimmon leaves using near-infrared spectroscopy (NIRS) in combination with multivariate calibration techniques. Based on a training dataset of 134 samples, a predictive model was developed from their NIR spectral data. For modelling, the partial least squares regression (PLSR) method was used. The best model was obtained with the first derivative of the apparent absorbance and using just 10 latent components. In the subsequent external validation carried out with 35 external data this model reached r 2 = 0.93, RMSE = 0.16 % and RPD = 3.6, with standard error of 0.026 % and bias of −0.05 %. From these results, the model based on NIR spectral readings can be used for speeding up the laboratory determination of chloride in persimmon leaves with only a modest loss of precision. The intermolecular interaction between chloride ions and the peptide bonds in leaf proteins through hydrogen bonding, i.e. N–H···Cl, explains the ability for chloride determinations on the basis of NIR spectra.
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spelling ReDivia65872025-04-25T14:47:25Z Determination of persimmon leaf chloride contents using near-infrared spectroscopy (NIRS) De-Paz, José M. Visconti, Fernando Chiaravalle, Mara Quinones, Ana Chemometrics/statistics N01 Agricultural engineering Chlorides Agriculture NIR spectroscopy Early diagnosis of specific chloride toxicity in persimmon trees requires the reliable and fast determination of the leaf chloride content, which is usually performed by means of a cumbersome, expensive and time-consuming wet analysis. A methodology has been developed in this study as an alternative to determine chloride in persimmon leaves using near-infrared spectroscopy (NIRS) in combination with multivariate calibration techniques. Based on a training dataset of 134 samples, a predictive model was developed from their NIR spectral data. For modelling, the partial least squares regression (PLSR) method was used. The best model was obtained with the first derivative of the apparent absorbance and using just 10 latent components. In the subsequent external validation carried out with 35 external data this model reached r 2 = 0.93, RMSE = 0.16 % and RPD = 3.6, with standard error of 0.026 % and bias of −0.05 %. From these results, the model based on NIR spectral readings can be used for speeding up the laboratory determination of chloride in persimmon leaves with only a modest loss of precision. The intermolecular interaction between chloride ions and the peptide bonds in leaf proteins through hydrogen bonding, i.e. N–H···Cl, explains the ability for chloride determinations on the basis of NIR spectra. 2020-09-02T08:37:06Z 2020-09-02T08:37:06Z 2016 publishedVersion de Paz, J. M., Visconti, F., Chiaravalle, M., & Quiñones, A. (2016). Determination of persimmon leaf chloride contents using near-infrared spectroscopy (NIRS). Analytical and Bioanalytical Chemistry, 408(13), 3537-3545. 1618-2642 http://hdl.handle.net/20.500.11939/6587 10.1007/s00216-016-9430-2 https://link.springer.com/article/10.1007%2Fs00216-016-9430-2 en Atribución-NoComercial-SinDerivadas 3.0 España http://creativecommons.org/licenses/by-nc-nd/3.0/es/ closedAccess Springer Verlag electronico
spellingShingle Chemometrics/statistics
N01 Agricultural engineering
Chlorides
Agriculture
NIR spectroscopy
De-Paz, José M.
Visconti, Fernando
Chiaravalle, Mara
Quinones, Ana
Determination of persimmon leaf chloride contents using near-infrared spectroscopy (NIRS)
title Determination of persimmon leaf chloride contents using near-infrared spectroscopy (NIRS)
title_full Determination of persimmon leaf chloride contents using near-infrared spectroscopy (NIRS)
title_fullStr Determination of persimmon leaf chloride contents using near-infrared spectroscopy (NIRS)
title_full_unstemmed Determination of persimmon leaf chloride contents using near-infrared spectroscopy (NIRS)
title_short Determination of persimmon leaf chloride contents using near-infrared spectroscopy (NIRS)
title_sort determination of persimmon leaf chloride contents using near infrared spectroscopy nirs
topic Chemometrics/statistics
N01 Agricultural engineering
Chlorides
Agriculture
NIR spectroscopy
url http://hdl.handle.net/20.500.11939/6587
https://link.springer.com/article/10.1007%2Fs00216-016-9430-2
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